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Nonlinear optics
Nonlinear optics (NLO) is a branch of optics that studies the case when optical properties of matter depend on the intensity of the input light. Nonlinear phenomena become relevant only when the input light is very intense. Typically, in order to observe nonlinear phenomena, an intensity of the electromagnetic field of light larger than 108 V/m (and thus comparable to the atomic electric field of ~1011 V/m) is required. In this case, the polarization density P responds non-linearly to the electric field E of light. In order to obtain an electromagnetic field that is sufficiently intense, laser sources must be used. In nonlinear optics, the superposition principle no longer holds, and the polarization of the material is no longer linear in the electric field intensity. Instead, in the perturbative limit, it can be expressed by a polynomial sum of order n. Many different physical mechanisms can cause nonlinearities in the optical behaviour of a material, i.e. the motion of bound electrons, field-induced vibrational or orientational motions, optically-induced acoustic waves and thermal effects. The motion of bound electrons, in particular, has a very short response timescale, so it is of particular relevance in the context of ultrafast nonlinear optics. The simplest way to picture this behaviour in a semiclassical way is to use a phenomenological model: an anharmonic oscillator can model the forced oscillations of a bound electron inside the medium. In this picture, the binding interaction between the ion core and the electron is the Coulomb force and nonlinearities appear as changes in the elastic constant of the system (which behaves similarly to a mass attached to a spring) when the stretching or compression of the oscillator is large enough.
It must be pointed out that Maxwell's equations are linear in vacuum, so, nonlinear processes only occur in media. However, the theory of quantum electrodynamics (QED) predicts that, above the Schwinger limit, vacuum itself can behave in a nonlinear way.
The description of nonlinear optics usually presented in textbooks is the perturbative regime, which is valid when the input intensity remains below 1014 W/cm2, which implies that the electric field is well below the intensity of interatomic fields. This approach allows to use a Taylor series to write down the polarization density as a polynomial sum. It is also possible to study the laser-matter interaction at a much higher intensity of light: this field is referred to as nonperturbational nonlinear optics or extreme nonlinear optics and investigates the generation of extremely high-order harmonics, attosecond pulse generation and relativistic nonlinear effects.
The first nonlinear optical effect to be predicted was two-photon absorption, by Maria Goeppert Mayer for her PhD in 1931, but it remained an unexplored theoretical curiosity until 1961 and the almost simultaneous observation of two-photon absorption at Bell Labs and the discovery of second-harmonic generation by Peter Franken et al. at University of Michigan, both shortly after the construction of the first laser by Theodore Maiman. However, some nonlinear effects were discovered before the development of the laser. The theoretical basis for many nonlinear processes was first described in Bloembergen's monograph "Nonlinear Optics".
Nonlinear optics explains nonlinear response of properties such as frequency, polarization, phase or path of incident light. These nonlinear interactions give rise to a host of optical phenomena:
In these processes, the medium has a linear response to the light, but the properties of the medium are affected by other causes:
Nonlinear effects fall into two qualitatively different categories, parametric and non-parametric effects. A parametric non-linearity is an interaction in which the quantum state of the nonlinear material is not changed by the interaction with the optical field. As a consequence of this, the process is "instantaneous". Energy and momentum are conserved in the optical field, making phase matching important and polarization-dependent.
Parametric and "instantaneous" (i.e. material must be lossless and dispersionless through the Kramers–Kronig relations) nonlinear optical phenomena, in which the optical fields are not too large, can be described by a Taylor series expansion of the dielectric polarization density (electric dipole moment per unit volume) P(t) at time t in terms of the electric field E(t):
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Nonlinear optics
Nonlinear optics (NLO) is a branch of optics that studies the case when optical properties of matter depend on the intensity of the input light. Nonlinear phenomena become relevant only when the input light is very intense. Typically, in order to observe nonlinear phenomena, an intensity of the electromagnetic field of light larger than 108 V/m (and thus comparable to the atomic electric field of ~1011 V/m) is required. In this case, the polarization density P responds non-linearly to the electric field E of light. In order to obtain an electromagnetic field that is sufficiently intense, laser sources must be used. In nonlinear optics, the superposition principle no longer holds, and the polarization of the material is no longer linear in the electric field intensity. Instead, in the perturbative limit, it can be expressed by a polynomial sum of order n. Many different physical mechanisms can cause nonlinearities in the optical behaviour of a material, i.e. the motion of bound electrons, field-induced vibrational or orientational motions, optically-induced acoustic waves and thermal effects. The motion of bound electrons, in particular, has a very short response timescale, so it is of particular relevance in the context of ultrafast nonlinear optics. The simplest way to picture this behaviour in a semiclassical way is to use a phenomenological model: an anharmonic oscillator can model the forced oscillations of a bound electron inside the medium. In this picture, the binding interaction between the ion core and the electron is the Coulomb force and nonlinearities appear as changes in the elastic constant of the system (which behaves similarly to a mass attached to a spring) when the stretching or compression of the oscillator is large enough.
It must be pointed out that Maxwell's equations are linear in vacuum, so, nonlinear processes only occur in media. However, the theory of quantum electrodynamics (QED) predicts that, above the Schwinger limit, vacuum itself can behave in a nonlinear way.
The description of nonlinear optics usually presented in textbooks is the perturbative regime, which is valid when the input intensity remains below 1014 W/cm2, which implies that the electric field is well below the intensity of interatomic fields. This approach allows to use a Taylor series to write down the polarization density as a polynomial sum. It is also possible to study the laser-matter interaction at a much higher intensity of light: this field is referred to as nonperturbational nonlinear optics or extreme nonlinear optics and investigates the generation of extremely high-order harmonics, attosecond pulse generation and relativistic nonlinear effects.
The first nonlinear optical effect to be predicted was two-photon absorption, by Maria Goeppert Mayer for her PhD in 1931, but it remained an unexplored theoretical curiosity until 1961 and the almost simultaneous observation of two-photon absorption at Bell Labs and the discovery of second-harmonic generation by Peter Franken et al. at University of Michigan, both shortly after the construction of the first laser by Theodore Maiman. However, some nonlinear effects were discovered before the development of the laser. The theoretical basis for many nonlinear processes was first described in Bloembergen's monograph "Nonlinear Optics".
Nonlinear optics explains nonlinear response of properties such as frequency, polarization, phase or path of incident light. These nonlinear interactions give rise to a host of optical phenomena:
In these processes, the medium has a linear response to the light, but the properties of the medium are affected by other causes:
Nonlinear effects fall into two qualitatively different categories, parametric and non-parametric effects. A parametric non-linearity is an interaction in which the quantum state of the nonlinear material is not changed by the interaction with the optical field. As a consequence of this, the process is "instantaneous". Energy and momentum are conserved in the optical field, making phase matching important and polarization-dependent.
Parametric and "instantaneous" (i.e. material must be lossless and dispersionless through the Kramers–Kronig relations) nonlinear optical phenomena, in which the optical fields are not too large, can be described by a Taylor series expansion of the dielectric polarization density (electric dipole moment per unit volume) P(t) at time t in terms of the electric field E(t):
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